Must play PS3 games on Premium

Hello, I just got an upgrade to my subscription as a surprise gift and now I want to dive in the games I never could.

PS3 is the only PlayStation generation that I missed and there's quite a few gems that I want to try. What are some of the best PS3 games on Premium that I should play?

I'm aiming at: God of War Ascension - it's literally the only GoW game I haven't played. Everything Ratchet & Clank on PS3. I'd add MGS 4, but I didn't see it there.

So any other PS3 game recommendations?

I've played the Uncharted remakes and The Last of Us.